Journal
ORGANIC LETTERS
Volume 14, Issue 5, Pages 1310-1313Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol300192p
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Funding
- Institute of Chemical Research of Catalonia (ICIQ) Foundation
- MICINN [CTQ2010-15513]
- European Union [FP7-PEOPLE-2010-IIF n: 273088]
- ICREA Funding Source: Custom
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Expanding upon the recently developed aminocatalytic asymmetric indole-2,3-quinodimethane strategy, a straightforward synthesis of structurally and stereochemically complex tetrahydrocarbazoles has been devised. The chemistry's complexity-generating power was further harnessed by designing a multicatalytic, one-pot Diels-Alder/benzoin reaction sequence to stereoselectively access trans-fused tetracyclic indole-based compounds having four stereogenic centers with very high fidelity.
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