Journal
ORGANIC LETTERS
Volume 14, Issue 10, Pages 2642-2645Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol301034j
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- UBE Foundation
- [24686092]
- Grants-in-Aid for Scientific Research [24686092] Funding Source: KAKEN
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A copper-catalyzed formic acid synthesis from CO2 with hydrosilanes has been accomplished. The Cu(OAc)(2)center dot H2O-1,2-bis(diphenylphosphino)benzene system is highly effective for the formic acid synthesis under 1 atm of CO2. The TON value approached 8100 in 6 h. The reaction pathway was revealed by in situ NMR analysis and isotopic experiments.
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