Journal
ORGANIC LETTERS
Volume 14, Issue 11, Pages 2846-2849Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol3010936
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Funding
- National Science Foundation [CHE-1112055]
- Russian Foundation for Basic Research (RFBR) [10-03-00370]
- Division Of Chemistry
- Direct For Mathematical & Physical Scien [1112055] Funding Source: National Science Foundation
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A general highly regio- and stereoselective palladium-catalyzed head-to-head dimerization reaction of terminal acetylenes is presented. This methodology allows for the efficient synthesis of a variety of 1,4-enynes as single E stereoisomers. Computational studies reveal that this dimerization reaction proceeds via the hydropalladation pathway.
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