Journal
ORGANIC LETTERS
Volume 14, Issue 11, Pages 2702-2705Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol300887t
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Funding
- MEXT
- JSPS
- Kuraray Co. Ltd.
- Grants-in-Aid for Scientific Research [23750113, 24106730, 23655085, 24105522] Funding Source: KAKEN
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The first synthesis of nitrogen-bridged terthiophenes (NBTTs) has been achieved by a tandem Buchwald-Hartwig coupling of 3,3',3 '', 4'-tetrabromo-2,2':5',2 ''-terthiophene. Several NBTT derivatives bearing aryl or alkyl moieties on the N-atoms could be synthesized. Their fundamental electrochemical characteristics and HOMO-LUMO levels were found to be influenced by the substituents on the N-atoms.
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