Journal
ORGANIC LETTERS
Volume 14, Issue 20, Pages 5210-5213Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol3023038
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Funding
- NSFC [20928001, 21232004, 21072163, 21002083, 21102124]
- PAPD of Jiangsu Higher Education Institutions
- Robert A. Welch Foundation [D-1361]
- NIH [R21DA031860-01]
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Efficient three-component domino strategies for the synthesis of multifunctionalized tetracyclic indeno[1,2-b]indole derivatives with different substituted patterns have been established successfully. The first pathway involves a novel sequential methyl migration, aromatization, and esterification, while a second reaction in HOAc leads to compounds 6 with high syn diastereoselectivity. Both reactions showed attractive features including mild conditions, convenient one-pot operation, short reaction times of 15-32 min, and excellent regio- and/or stereoselectivity.
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