Journal
ORGANIC LETTERS
Volume 14, Issue 3, Pages 816-819Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol2033465
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Funding
- JSPS [21350020, 21750086]
- China Scholarship Council
- Grants-in-Aid for Scientific Research [21750086, 21350020] Funding Source: KAKEN
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A Cu-catalyzed gamma-selective coupling reaction between propargylic phosphates and aryl- or alkenylboronates afforded aryl- or alkenyl-conjugated allenes. The reaction showed excellent functional group compatibility in both the propargylic substrates and the boronates. The reaction of an enantioenriched propargylic phosphate proceeded with excellent chirality transfer with 1,3-anti stereochemistry to give axially chiral aryl- and alkenylallenes.
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