Journal
ORGANIC LETTERS
Volume 14, Issue 20, Pages 5350-5353Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol302535r
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Funding
- NIH [NIGMS RO1 08637]
- National Science Foundation
- Berkeley EDGE summer fellowship
- UC Berkeley for a Chancellor's Fellowship
- Eli Lilly
- Abbott
- Amgen
- Dupont
- Astra Zeneca
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An effective synthesis of the pentacyclic core of the unusual Kopsia alkaloid arboflorine is reported. The success of the synthetic route rested on the use of a borylative C-H functionalization reaction, a convergent Suzuki cross-coupling to a C(2) halogenated indole, and an unprecedented transannular dehydrogenative C-N bond forming reaction.
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