Journal
ORGANIC LETTERS
Volume 14, Issue 18, Pages 4794-4797Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol3020946
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Funding
- Ministry of Education, Culture, Sports, Science, and Technology, Japan
- Grants-in-Aid for Scientific Research [21106005, 23655035, 23350017, 21106001] Funding Source: KAKEN
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An efficient protocol for the aza-Diels-Alder reaction of electron-deficient 1,3-dienes with unactivated imines in the presence of a cationic cobalt(III) porphyrin complex was developed. The transformation proceeded smoothly to afford the desired piperidine scaffold within 2 h at ambient temperature. Highly chemoselective cycloaddition of imines with dienes in the presence of a variety of carbonyl compounds was also demonstrated.
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