Journal
ORGANIC LETTERS
Volume 13, Issue 3, Pages 434-437Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol102767j
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- National Institute of General Medical Sciences, National Institutes of Health [GM083944-03]
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This paper describes the regioselective diamination of conjugated dienes using inexpensive Cup) as catalyst and N,N-di-tert-butylthiadiaziridine 1,1-dioxide as nitrogen source. The regioselectivity of diamination is likely due to dual mechanistic pathways which are greatly influenced by reaction conditions and the nature of the diene. A variety of useful internal and terminal cyclic sulfamides can be obtained in good yield.
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