Journal
ORGANIC LETTERS
Volume 13, Issue 6, Pages 1338-1341Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol200006e
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Funding
- National Science Council, Taiwan, ROC
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A synthesis of fully substituted cyclopentanes bearing a quaternary carbon center and five contiguous stereogenic centers has been achieved by sequential organocatalyzed Stetter and Michael Aldol reactions of heteroaromatic aldehydes, nitroalkenes, and alpha,beta-unsaturated aldehydes via the [1 + 2 + 2] annulation strategy with dynamic kinetic asymmetric transformation and excellent enantioselectivities (up to > 99% ee).
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