Journal
ORGANIC LETTERS
Volume 12, Issue 22, Pages 5214-5217Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol102252n
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Funding
- National Natural Science Foundation of China [20872059, 21072091]
- MOST of China [2011CB808600]
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A novel cross dehydrogenative coupling (CDC) reaction of N,N-dimethylanilines with methyl ketones by cooperative copper and aminocatalysis has been developed, which leads to the formation of beta-arylamino ketones in 42-73% yields. Moreover, the copper-catalyzed alkylation of free (NH) indoles with N,N-dimethylanilines via CDC reaction is also presented, affording alkylated indoles in 52-78% yields.
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