Journal
ORGANIC LETTERS
Volume 12, Issue 19, Pages 4356-4359Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol101817g
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Funding
- Major State Basic Research Development Program [2009CB125905]
- National Natural Science Foundation of China [30870083, 31070051]
- Department of Science and Technology of Yunnan Province [2008CD068]
- Scientific Research Foundation for the Returned Overseas Chinese Scholars, State Education Ministry [[2009]1341]
- 12th Young Academic and Technical Leader Raising Foundation of Yunnan Province [2009CI051]
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The putative key biosynthetic intermediates of prenylated indole alkaloids have long been proposed but never isolated. Two such alkaloids, named talathermophilins A and B (1 and 2), were isolated from a thermophilic fungus Talaromyces thermophilus strain YM1-3 and were identified by NMR and MS spectroscopic analyses. The ratio of 1 and 2 in the culture broths was unexpectedly rather constant (about 2:3), which even remained unchanged despite the addition of exogenous 1 or 2, suggesting that talathermophilins might be of special function for the extremophilic fungus.
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