Journal
ORGANIC LETTERS
Volume 12, Issue 10, Pages 2194-2197Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol100474b
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Funding
- Hong Kong Research Grant Council
- GRF
- HKBU [202408]
- Hong Kong Baptist University
- Faculty Research Grant
- Research Grants Council of Hong Kong
- Consulate General of France in Hong Kong [F-HK04/07T]
- [FRG/08-09/11-16]
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A series of cyanine fluorophores based on fused aromatics as an electron donor for DNA sensing and two-photon bioimaging were synthesized, among which the carbazole-based biscyanine exhibits high sensitivity and efficiency as a fluorescent light-up probe for dsDNA, which shows selective binding toward the AT-rich regions. The synergetic effect of the bischromophoric skeleton gives a several-fold enhancement in a two-photon absorption cross-section as well as a 25- to 100-fold enhancement in two-photon excited fluorescence upon dsDNA binding.
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