Journal
ORGANIC LETTERS
Volume 12, Issue 20, Pages 4658-4660Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol101944j
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Asymmetric copper-catalyzed allylic substitution with methylmagnesium bromide is employed in combination with ring-closing olefin metathesis or ene-yne metathesis to achieve the synthesis of chiral, unsaturated nitrogen heterocycles. The resulting six- to eight-membered chiral heterocycles are accessible in high yields and with excellent enantioselectivities.
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