Journal
ORGANIC LETTERS
Volume 12, Issue 12, Pages 2806-2809Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol100895d
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Funding
- EPSRC
- BBSRC
- GlaxoSmithKline
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The regio- and stereoselective synthesis and subsequent Hiyama cross coupling of pentafluorophenyldimethylvinylsilanes has been developed, thus providing a convenient and robust method for the diversity-oriented synthesis of (E)-, (Z)- and alpha-disubstituted alkenes from terminal alkynes. Pentafluorophenyldimethylvinylsilanes undergo cross-coupling reactions with excellent selectivity and in good yields, offering an attractive alternative to existing masked silanols.
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