Journal
ORGANIC LETTERS
Volume 11, Issue 14, Pages 3028-3031Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol901041n
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Funding
- NUS Young Investigator Award [R-143-000-356-101]
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A series of triphenylene and trinaphthylene carboximides were synthesized mainly through Diels-Alder reactions between the in situ generated radialenes and N-alkylmaleimides. High electron affinity was obtained due to the attachment of electron-withdrawing carboximide groups. These disklike molecules can assemble into one-dimensional columnar structures in solid state and their mesophase properties were characterized by DSC, POM, and X-ray diffraction. Long-range ordered columnar phase was observed, qualifying them as potential n-type semiconductors in electronic devices.
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