Journal
ORGANIC LETTERS
Volume 11, Issue 6, Pages 1425-1428Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol900090f
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Funding
- National Natural Science Foundation of China [20702006]
- Shanghai Rising-Star program [07QA14007]
- Fudan University
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An efficient transition-metal-free intermolecular benzylic amidation with sulfonamides is described. Various valuable nitrogen-containing compounds, including amines, beta-chloro amine, amino alcohol, alpha-, beta-amino ester, and N-sulfonyl imine, are generated from the preferential N-functionalization of saturated benzylic C-H bonds. The potential of this reaction system also lies in the fact it can be developed into an environmentally friendly intermolecular amidation process.
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