Journal
ORGANIC LETTERS
Volume 11, Issue 9, Pages 2019-2022Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol900481e
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- Natural Sciences and Engineering Research Council of Canada (NSERC)
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An efficient method for the rapid construction of carbo- and heterocycles has been developed using radical relay cyclizations initiated by alkoxy radicals. Linear substrates were cyclized to form a wide range of cyclopentane, pyrrolidine, tetrahydropyran, and tetrahydrofuran derivatives in excellent yields. This methodology was utilized as a key step in the synthesis of the tetrahydrofuran fragment in (-)-amphidinolide K.
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