Journal
ORGANIC LETTERS
Volume 11, Issue 15, Pages 3378-3381Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol901221q
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Funding
- SRC (KOSEF) [R11-2005-008-00000-0]
- MEST
- KOSEF [R01-2006-10696]
- Korea Institute of Science and Technology Information [KSC-2007-S00-0018]
- National Research Foundation of Korea [과09A1514, 2009-0081566, 2008-0057799] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
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Synthesis of a novel pyrene derivative sensor (1) and its intermolecular binding pattern to Cu2+ in CH3CN were investigated. Upon Cu2+ binding, the sensor exhibited a strong static excimer emission at 460 nm, along with a weak monomer emission at 388 nm. The excimer emission intensity induced by the Cu2+ ion declined as the spacer length between the pyrene and quinolinylamide unit increased. The Cu2+ ion-induced self-assembled pyrenyl excimer formation is rationalized by fluorescence experiments and theoretical DFT calculations.
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