Journal
ORGANIC LETTERS
Volume 11, Issue 18, Pages 4116-4119Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol901614t
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Funding
- DFG [SPP1179]
- Fonds der Chemischen Industrie
- Alexander von Humboldt Foundation
- Aragon I+D Foundation
- Spanish Ministry of Science and Innovation
- CSIC [PIE 2008801260]
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The intramolecular Rauhut-Currier reaction creates a carbon-carbon bond between two tethered Michael acceptors. Previous asymmetric versions have relied on 1,4-additions of chiral nucleophilic catalysts. Herein, we investigate a novel strategy that involves the formation of electron rich dienamines as key intermediates. Our methodology provides an efficient entry to the iridoid framework.
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