Journal
ORGANIC LETTERS
Volume 11, Issue 15, Pages 3226-3229Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol9012469
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Funding
- National Natural Science Foundation of China [20802076, 20873145]
- Chinese Academy of Sciences [DICP-S200802]
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A new class of chiral ferrocenyl diphosphine ligands with an imidazole ring, (R-c, S-Fc)-ImiFerroPhos, has been prepared from acylferrocenes through a five-step transformation and successfully applied in the Rh-catalyzed asymmetric hydrogenation of various 3-aryl-substituted 2-phosphonomethylpropenoates, in which a series of chiral 3-phosphono-2-arylmethylpropanoic acid derivatives were achieved in ee values of up to 98%.
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