Journal
ORGANIC LETTERS
Volume 11, Issue 23, Pages 5410-5412Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol902270f
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Funding
- Deutsche Forschungsgemeinschaft (DFG)
- Dr. Philipp Heretsch is a fellow of Fonds der Chemischen Industric
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All four diastereomers of the trisubstituted piperidine-alkaloids of the veratramine and jervine type were synthesized with complete stereocontrol starting from enantiopure citronellic acids. The flexible, high-yielding, and scalable route described here will facilitate convergent syntheses and give access to analogues of cyclopamine and other biologically active and diverse steroid alkaloids.
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