Journal
ORGANIC LETTERS
Volume 10, Issue 7, Pages 1437-1440Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol800259s
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The first total synthesis of the indole alkaloid mersicarpine is reported. Key steps include a beta-dicarbonyl radical cyclization, as well as an oxidation of the benzopyrrole moiety to establish the masked 1,2-dicarbonyl functionality. An X-ray crystal structure and discussion of the (1)H NMR behavior of the natural product are also presented.
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