Journal
ORGANIC LETTERS
Volume 10, Issue 8, Pages 1541-1544Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol800242n
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Funding
- NIGMS NIH HHS [S06 GM008136, S06 GM008136-320042] Funding Source: Medline
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The synthesis of naphthalene derivatives through three-component coupling of 2-alkynylbenzaidehyde hydrazones with carbene complexes and electron-deficient alkynes has been examined. The reaction involves formation of an isoindole derivative, followed by intramolecular Diels-Alder reaction, followed by nitrene extrusion. The reaction was highly regioselective using unsymmetrical alkynes.
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