Journal
ORGANIC LETTERS
Volume 10, Issue 19, Pages 4159-4162Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol801416n
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The concept of cyanine has been successfully extended to an anionic heptamethine dye featuring tricyanofuran (TCF) moieties in terms of structure, reactivity, and photophysical properties. Importantly, absorption and emission are red-shifted compared to its classical cationic analog without any cost in terms of thermal stability. In addition to its cyanine behavior, this molecule exhibits further redox properties: oxidation and reduction led to the reversible formation of radical species whose absorption is in marked contrast with that of cyanines.
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