Journal
ORGANIC ELECTRONICS
Volume 63, Issue -, Pages 398-414Publisher
ELSEVIER
DOI: 10.1016/j.orgel.2018.09.010
Keywords
Polymer semiconductors; Organic electronics; Device physics; Organic electrochemical transistors; Thin-film transistors
Funding
- National Science Foundation Graduate Research Fellowship [DGE 1144083]
- NSF [NSF EPMD 1509909]
- Graduate Assistantships in Areas of National Need Award [P200A120063]
- NSF GRFP [DGE 1144083]
- National Science Foundation Grant CAREER [0847390]
- National Science Foundation [ECCS 1509909]
- Division Of Materials Research
- Direct For Mathematical & Physical Scien [0847390] Funding Source: National Science Foundation
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Organic electrochemical transistors (OECTs) are thin-film transistors that have shown great promise in a range of applications including biosensing, logic circuits, and neuromorphic engineering. The device physics of OECTs are determined by the interaction between ionic and electronic charge carriers. This interaction sets OECTs apart from conventional transistor technologies and has necessitated the development of device models for the unique behavior of OECTs. In this Review, we discuss existing models for OECTs and provide a framework for understanding these models. Moreover, we show how the insight from these models inform device optimization. Finally, we discuss details of OECT operation that are not well-understood and that provide exciting opportunities for future research.
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