Journal
ORGANIC & BIOMOLECULAR CHEMISTRY
Volume 10, Issue 27, Pages 5307-5314Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c2ob25469g
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Funding
- National Natural Science Foundation of China [30925039]
- Beijing Natural Science Foundation [5111003]
- Ministry of Science and Technology of China [2010ZX09401-403, 2012ZX09301-003]
- Chinese Academy of Sciences [KSCX2-EW-G-6]
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Natural products possessing the 3-(furan-2(5H)-ylidene)furan-2,4(3H,5H)-dione (furylidene tetronic acid) skeleton are rare and were encountered only as fungal metabolites. The configurational assignment of the furylidene tetronic acid core using conventional approaches remained a challenge. Pestalotic acids A-G (1-7) are new furylidene tetronic acid derivatives isolated from a plant endophyte Pestalotiopsis yunnanensis. The structure of 1 was elucidated by combination of NMR experiments, X-ray crystallography, and ECD calculations. Compounds 3 and 7 showed significant antimicrobial activity.
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