Journal
ORGANIC & BIOMOLECULAR CHEMISTRY
Volume 10, Issue 29, Pages 5629-5635Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c2ob25489a
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A synthesis of the core ring structure of the fargenin/fargenone family of natural products is presented. The general strategy is based upon biosynthetic speculation and exploits a cascade reaction, which transforms a spirocyclic dienone into the core ring system via a deprotonation-oxy-Michael-Wittig olefination sequence. This study represents the first synthesis work towards this family of natural products.
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