Journal
ORGANIC & BIOMOLECULAR CHEMISTRY
Volume 9, Issue 3, Pages 667-669Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c0ob00914h
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Funding
- Irish Research Council for Science, Engineering and Technology
- Eli Lilly
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Asymmetric copper-catalysed intramolecular C-H insertion reactions of a series of alpha-diazo-beta-keto sulfones are reported. Enantioselectivities of up to 82% ee were achieved in moderate to good yield. These results represent the highest level of enantiocontrol achieved to date for a copper-catalysed cyclopentanone synthesis via C-H insertion.
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