Journal
ORGANIC & BIOMOLECULAR CHEMISTRY
Volume 8, Issue 20, Pages 4767-4774Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c0ob00154f
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Funding
- National Natural Science Foundation of China [20902018]
- Shanghai Pujiang Program [08PJ1403300]
- Fundamental Research Funds for the Central Universities
- 111 Project [B07023]
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The first highly efficient Michael addition of challenging alpha,alpha-disubstituted aldehydes to maleimides catalyzed by a simple bifunctional primary amine thiourea catalyst/benzoic acid system has been successfully developed to generate quaternary carbon centers in high yields (up to 99%) with excellent enantioselectivities (91-99%).
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