Journal
OPTICS LETTERS
Volume 35, Issue 21, Pages 3664-3666Publisher
OPTICAL SOC AMER
DOI: 10.1364/OL.35.003664
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- United States Department of Energy (DOE) Office of Basic Energy Sciences [AC02-05CH1123, DE-FG-52-06NA26212]
- Fannie and John Hertz Foundation
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We combine different wavelengths from an intense high-order harmonics source with variable delay at the focus of a split-mirror interferometer to conduct pump-probe experiments on gas-phase molecules. We report measurements of the time resolution (<44 fs) and spatial profiles (4 mu m x 12 mu m) at the focus of the apparatus. We demonstrate the utility of this two-color, high-order-harmonic technique by time resolving molecular hydrogen elimination from C(2)H(4) excited into its absorption band at 161 nm. (C) 2010 Optical Society of America
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