Journal
OPTICS LETTERS
Volume 33, Issue 18, Pages 2086-2088Publisher
OPTICAL SOC AMER
DOI: 10.1364/OL.33.002086
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Funding
- Swiss National Science Foundation [200021-111902/1]
- University of Zurich
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We present an experimental setup to detect transient vibrational circular dichroism signals. A femtosecond laser system is synchronized to a photoelastic modulator to produce alternating left- and right-handed circularly polarized mid-IR pulses at 1 kHz repetition rate. Transient changes in the circular dichroism of the CH-stretch vibrations of a cobalt-sparteine complex were probed in a proof-of-principle experiment and are clearly distinct from conventional transient absorption changes. (C) 2008 Optical Society of America
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