Journal
OPTICS EXPRESS
Volume 19, Issue 6, Pages 5528-5535Publisher
OPTICAL SOC AMER
DOI: 10.1364/OE.19.005528
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Funding
- National Science Foundation [CMMI-0729263, ECCS-0846818, ECCS-0824186]
- Army Research Office [49653-EL, DURIP 2008-02-136]
- Directorate For Engineering
- Div Of Electrical, Commun & Cyber Sys [0824186, 0846818] Funding Source: National Science Foundation
- Div Of Industrial Innovation & Partnersh
- Directorate For Engineering [1010491] Funding Source: National Science Foundation
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High-quality InP/ZnS core-shell nanocrystal quantum dots (NQDs) were synthesized as a heavy-metal-free alternative to the gain media of cadmium-based colloidal nanoparticles. Upon UV excitation, amplified spontaneous emission (ASE) and optical gain were observed, for the first time, in close-packed InP/ZnS core-shell NQDs. The ASE wavelength can be selected by tailoring the nanocrystal size over a broad range of the spectrum. Moreover, the optical gain profile of InP/ZnS NQDs was matched to the second order feedback of holographic polymer-dispersed liquid crystal gratings, leading to the very first demonstration of an optically-pumped, nanocrystal laser based on InP/ZnS core-shell NQDs. (C) 2011 Optical Society of America
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