Journal
OPTICS EXPRESS
Volume 18, Issue 17, Pages 17699-17708Publisher
OPTICAL SOC AMER
DOI: 10.1364/OE.18.017699
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Funding
- National Science Foundation
- Chemical Sciences, Geosciences, and Biosciences Division Office of Basic Energy Sciences, U.S. Department of Energy
- National Academy of Sciences/National Research Council
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We derive an analytical form for resonance lineshapes in two-dimensional (2D) Fourier transform spectroscopy. Our starting point is the solution of the optical Bloch equations for a two-level system in the 2D time domain. Application of the projection-slice theorem of 2D Fourier transforms reveals the form of diagonal and cross-diagonal slices in the 2D frequency data for arbitrary inhomogeneity. The results are applied in quantitative measurements of homogeneous and inhomogeneous broadening of multiple resonances in experimental data. (C) 2010 Optical Society of America
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