Journal
OPTICS EXPRESS
Volume 16, Issue 22, Pages 17420-17428Publisher
OPTICAL SOC AMER
DOI: 10.1364/OE.16.017420
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Funding
- Office of Basic Energy Sciences
- US Department of Energy
- American Chemical Society Petroleum Research Fund
- Alfred P. Sloan Foundation
- National Science Foundation
- Division Of Physics
- Direct For Mathematical & Physical Scien [0748470] Funding Source: National Science Foundation
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We report two-color two-dimensional Fourier transform electronic spectroscopy obtained using an acousto-optic pulse-shaper in a pump-probe geometry. The two-color setup will facilitate the study of energy transfer between electronic transitions that are widely separated in energy. We demonstrate the method at visible wavelengths on the laser dye LDS750 in acetonitrile. We discuss phase-cycling and polarization schemes to optimize the signal-to-noise ratio in the pump-probe geometry. We also demonstrate that phase-cycling can be used to separate rephasing and nonrephasing signal components. (C) 2008 Optical Society of America
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