Journal
OPTICS EXPRESS
Volume 17, Issue 1, Pages 248-259Publisher
OPTICAL SOC AMER
DOI: 10.1364/OE.17.000248
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Funding
- UK NERC Molecular Spectroscopy Facility
- MIRTHE NSF Engineering Research Center
- Aerodyne Research Inc
- RAL Space Science and Technology Department (SSTD)
- Natural Environment Research Council [MSF010001] Funding Source: researchfish
- NERC [MSF010001] Funding Source: UKRI
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Broadband thermal infrared heterodyne spectro-radiometry using an external cavity quantum cascade laser as a tunable local oscillator has been performed over a frequency range of more than 100 cm(-1) at a central frequency of 1190 cm(-1). Heterodyne spectro-radiometry is demonstrated for two local oscillator tuning modes: broadband tuning for transmission and emission spectroscopy of broadband absorbers (Freon 12), and broadband frequency selection in combination with fine continuous frequency tuning for high- resolution (0.021 cm(-1)) transmission spectroscopy (N2O). In each case concentration retrievals are performed and analyzed. The spectroradiometer noise level is demonstrated to be twenty two and eight times the fundamental shot-noise limit in the two scanning modes respectively. (C) 2008 Optical Society of America
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