4.6 Article

All-optical retrieval of the global phase for two-dimensional Fourier-transform spectroscopy

Journal

OPTICS EXPRESS
Volume 16, Issue 22, Pages 18017-18027

Publisher

OPTICAL SOC AMER
DOI: 10.1364/OE.16.018017

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Funding

  1. NSF
  2. Chemical Sciences, Geosciences, and Biosciences Division Office of Basic Energy Sciences, U.S. Department of Energy

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A combination of spatial interference patterns and spectral interferometry are used to find the global phase for non-collinear two-dimensional Fourier-transform (2DFT) spectra. Results are compared with those using the spectrally resolved transient absorption (STRA) method to find the global phase when excitation is with co-linear polarization. Additionally cross-linear polarized 2DFT spectra are correctly phased using the all-optical technique, where the SRTA is not applicable. (C) 2008 Optical Society of America

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