Journal
TETRAHEDRON
Volume 71, Issue 23, Pages 4035-4038Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.tet.2015.04.058
Keywords
Rh(I)-catalyzed; Carbazoles; C-N cleavage; Decarbonylation
Categories
Funding
- National Natural Science Foundation of China [21302066]
- Young Program, SCF of Jiangsu Province [BK20130129]
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A one-pot Rh(I)-catalyzed synthesis of 9-H carbazoles via C-N bond cleavage by activation of aldehyde C-H bonds is reported. This protocol offers good yields and tolerates a broad range of functional groups. Based on the extensive control experiments, we propose a plausible decarbonylation mechanism. (C) 2015 Elsevier Ltd. All rights reserved.
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