Journal
SYNLETT
Volume 27, Issue 3, Pages 331-336Publisher
GEORG THIEME VERLAG KG
DOI: 10.1055/s-0035-1561282
Keywords
dehydrogenation; oxidation; catalysis; palladium; allyl complexes
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Funding
- Yale University
- NSF [DGE-1122492]
- Anderson Foundation
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Palladium-allyl chemistry has historically been used as a means of allylation of nucleophiles, as developed by Tsuji and Trost in the 1970s. Also during this decade, the Saegusa oxidation, the most prominent palladium-catalyzed dehydrogenation reaction, was developed. This Synpacts article provides a historical overview of dehydrogenation adjacent to carbonyls and our recent contribution to this area: palladium-allyl catalyzed dehydrogenation of nitriles and esters.
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