4.6 Article

Atomic photoionization in combined intense XUV free-electron and infrared laser fields

Journal

NEW JOURNAL OF PHYSICS
Volume 14, Issue -, Pages -

Publisher

IOP PUBLISHING LTD
DOI: 10.1088/1367-2630/14/4/043008

Keywords

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Funding

  1. DFG [SFB 652/2]
  2. EU RTD [HRPI-CT-1999-50009]
  3. Science Foundation Ireland [07/IN.1/I1771]
  4. HEA PRTLI IV and V INSPIRE
  5. IRCSET (Irish Research Council for Science, Engineering and Technology)
  6. France-Ireland ULYSSES
  7. National Nature Science Foundation of China [11075118]

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We present a systematic study of the photoionization of noble gas atoms exposed simultaneously to ultrashort (20 fs) monochromatic (1-2% spectral width) extreme ultraviolet (XUV) radiation from the Free-electron Laser in Hamburg (FLASH) and to intense synchronized near-infrared (NIR) laser pulses with intensities up to about 10(13) W cm(-2). Already at modest intensities of the NIR dressing field, the XUV-induced photoionization lines are split into a sequence of peaks due to the emission or absorption of several additional infrared photons. We observed a plateau-shaped envelope of the resulting sequence of sidebands that broadens with increasing intensity of the NIR dressing field. All individual lines of the nonlinear two-color ionization process are Stark-shifted, reflecting the effective intensity of the NIR field. The intensity-dependent cutoff energies of the sideband plateau are in good agreement with a classical model. The detailed structure of the two-color spectra, including the formation of individual sidebands, the Stark shifts and the contributions beyond the classical cut-off, however, requires a fully quantum mechanical description, as is demonstrated with time-dependent quantum calculations in single-active electron approximation.

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