Journal
NEW JOURNAL OF CHEMISTRY
Volume 37, Issue 11, Pages 3402-3405Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3nj00276d
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Funding
- Center for Electrocatalysis, Transport Phenomena, and Materials (CETM) for Innovative Energy Storage, an Energy Frontier Research Center
- U.S. Department of Energy, Office of Basic Energy Sciences [DE-SC00001055]
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We now report the electrocatalytic dehydrogenation of tetra-hydroquinaldine by an electron-rich CpNi N-heterocyclic carbene (NHC) with quinoid ligand motifs and explore the effects of quinone additives on CpNi compounds without quinoid NHC ligands. Our CpNi(NHC) catalyst exhibits dehydrogenative electrocatalytic activity and demonstrates that a molecular catalyst precursor can be viable in the electrode-driven (H+ + e(-)) release step of virtual hydrogen storage''.
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