4.6 Article

Effect of fluid-colloid interactions on the mobility of a thermophoretic microswimmer in non-ideal fluids

Journal

SOFT MATTER
Volume 11, Issue 33, Pages 6703-6715

Publisher

ROYAL SOC CHEMISTRY
DOI: 10.1039/c5sm01364j

Keywords

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Funding

  1. Alexander von Humboldt Foundation
  2. Julich Supercomputing Center
  3. Deutsche Forschungsgemeinschaft

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Janus colloids propelled by light, e.g., thermophoretic particles, offer promising prospects as artificial microswimmers. However, their swimming behavior and its dependence on fluid properties and fluid-colloid interactions remain poorly understood. Here, we investigate the behavior of a thermophoretic Janus colloid in its own temperature gradient using numerical simulations. The dissipative particle dynamics method with energy conservation is used to investigate the behavior in non-ideal and ideal-gas like fluids for different fluid-colloid interactions, boundary conditions, and temperature-controlling strategies. The fluid-colloid interactions appear to have a strong effect on the colloid behavior, since they directly affect heat exchange between the colloid surface and the fluid. The simulation results show that a reduction of the heat exchange at the fluid-colloid interface leads to an enhancement of colloid's thermophoretic mobility. The colloid behavior is found to be different in non-ideal and ideal fluids, suggesting that fluid compressibility plays a significant role. The flow field around the colloid surface is found to be dominated by a source-dipole, in agreement with the recent theoretical and simulation predictions. Finally, different temperature-control strategies do not appear to have a strong effect on the colloid's swimming velocity.

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