Journal
NATURE PHYSICS
Volume 5, Issue 5, Pages 357-362Publisher
NATURE PUBLISHING GROUP
DOI: 10.1038/NPHYS1250
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Funding
- Welch foundation [A-1562]
- Airforce Office of Scientific Research AFOSR
- Sofja Kovalevskaja Award of the Alexander von Humboldt Foundation
- DFG Cluster of Excellence: Munich Centre for Advanced Photonics
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Full characterization of single ultrashort laser pulses, as needed for attosecond metrology and spectroscopy, requires precise measurement of the offset between the electric field and pulse envelope, or carrier-envelope phase (CEP). Until now, all CEP measurements have been made by averaging over a large number of phase-stabilized laser pulses. Here, we demonstrate the first single-shot CEP measurement of intense few-cycle laser pulses. We focus a laser pulse on a gas target and detect photoelectrons emitted in opposing directions ('left-right') parallel to the polarization of the laser. By comparing the left-right asymmetries of photoelectrons at different energies, we mapped the CEP of consecutive non-phase-stabilized pulses on a parametric plot. This new evaluation method enables us to determine the CEP without phase ambiguity at unprecedented measurement precision. Future investigation of phase-dependent phenomena with CEP tagging at a much lower phase jitter than accessible at present with phase-stabilized lasers is now possible.
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