4.8 Article

Resonantly driven coherent oscillations in a solid-state quantum emitter

Journal

NATURE PHYSICS
Volume 5, Issue 3, Pages 203-207

Publisher

NATURE PUBLISHING GROUP
DOI: 10.1038/NPHYS1184

Keywords

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Funding

  1. National Science Foundation NSF-FRG [DMR-0606485]
  2. NSF-IGERT [DGE-0549417]
  3. Texas Advanced Research Program
  4. Direct For Mathematical & Physical Scien
  5. Division Of Materials Research [0906025] Funding Source: National Science Foundation

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Single-quantum emitters emit only one photon at a time(1,2), but the properties of the photon depend on how the emitter is excited(3). Incoherent excitation is simple and broadly used with solid-state emitters such as quantum dots, but does not allow direct manipulation of the quantum state. Coherent, resonant excitation on the other hand is used in pump-probe techniques to examine the quantum state of the emitter(4), but does not permit collection of the single-photon emission. Coherent control with simultaneous generation of photons has been an elusive goal in solid-state approaches, where, because of strong laser scattering at the detection wavelength, measurement of resonant emission has been limited to cross-polarized detection(5) or Stokes-shift techniques(6,7). Here we demonstrate that a semiconductor quantum dot in a microcavity can be resonantly driven and its single-photon emission extracted background free. Under strong continuous-wave excitation, the dot undergoes several Rabi oscillations before emitting, which are visible as oscillations in the second-order correlation function. The quantum-dot states are therefore 'dressed', resulting in a Mollow-triplet emission spectrum. Such coherent control will be necessary for future high-efficiency sources of indistinguishable single photons(3,8), which can be used for quantum key distribution(9) or through post-selection(10) to generate entangled photon pairs(11,12).

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