4.8 Article

Ultrahigh mobility and giant magnetoresistance in the Dirac semimetal Cd3As2

Journal

NATURE MATERIALS
Volume 14, Issue 3, Pages 280-284

Publisher

NATURE PUBLISHING GROUP
DOI: 10.1038/nmat4143

Keywords

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Funding

  1. Army Research Office (ARO) [W911NF-11-1-0379]
  2. MURI grant on Topological Insulators (ARO) [W911NF-12-1-0461]
  3. US National Science Foundation [DMR 0819860]
  4. Japan Student Services Organization
  5. National Science Foundation Cooperative Agreement, the State of Florida [DMR-1157490]
  6. US Department of Energy

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Dirac and Weyl semimetals are 3D analogues of graphene in which crystalline symmetry protects the nodes against gap formation(1-3). Na3Bi and Cd3As2 were predicted to be Dirac semimetals(4,5), and recently confirmed to be so by photoemission experiments(6-8). Several novel transport properties in a magnetic field have been proposed for Dirac semimetals(2,9-11). Here, we report a property of Cd3As2 that was unpredicted, namely a remarkable protection mechanism that strongly suppresses backscattering in zero magnetic field. In single crystals, the protection results in ultrahigh mobility, 9 x 10(6) cm(2) V-1 s(-1) at 5 K. Suppression of backscattering results in a transport lifetime 10(4) times longer than the quantum lifetime. The lifting of this protection by the applied magnetic field leads to a very large magnetoresistance. We discuss how this may relate to changes to the Fermi surface induced by the applied magnetic field.

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