Journal
NATURE MATERIALS
Volume 8, Issue 5, Pages 410-414Publisher
NATURE PUBLISHING GROUP
DOI: 10.1038/NMAT2431
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Funding
- NSF DMR [DMR-0704045]
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Microstructure evolution in complex nonlinear systems is of great interest from both scientific and engineering viewpoints. Here, we consider an important case of such an evolution, a coherent decomposition of a homogeneous parent phase involving the symmetry-lifting crystal lattice rearrangement of the product phase. It is shown that under certain conditions the transformation develops as a pseudospinodal decomposition, which is defined as a transformation with continuous changes of the compositions of both decomposed phases towards their equilibrium values. The pseudospinodal decomposition starts by the formation of a nanodomain precursor state with a so-called tweed structure. The three-dimensional modelling demonstrates that this tweed structure has an underlying chessboard feature, and this arrangement is a template for the further microstructure development that eventually produces a coherent two-phase chessboard nanowire pattern. The proposed theory and modelling describe the mechanism of the pseudospinodal decomposition and predict all observed three-dimensional features of the chessboard structure.
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