Journal
NATURAL PRODUCT REPORTS
Volume 28, Issue 4, Pages 763-782Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c0np00053a
Keywords
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Funding
- Agence Nationale pour la Recherche [A.N.R.-09-JCJC-0036]
- C.N.R.S.
- Universite Paul Cezanne [UMR 6263]
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Polycyclic structures fused at a central carbon are of great interest due to their appealing conformational features and their structural implications in biological systems. Although progress in the development of synthetic methodologies towards such structures has been impressive, the stereoselective construction of such quaternary stereocentres remains a significant challenge in the total synthesis of natural products. This review highlights the progress in the formation of 1-oxaspiro[4.n]alkan-2-ones (2 <= n <= 7) with concomitant formation of the quaternary spiro centre.
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