Journal
NANOSCALE
Volume 10, Issue 9, Pages 4173-4178Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c7nr09126e
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Funding
- National Key Research and Development Program of China [2017YFB0403601]
- National Natural Science Foundation of China [61675086, 61475062, 61722504, 51702115, 51772123]
- China Postdoctoral Science Foundation [2017M611319]
- National Postdoctoral Program for Innovative Talents [BX201600060]
- BORSF RCS, Institutional Development Award [P20GM103424]
- Open Research Fund of State Key Laboratory of Polymer Physics and Chemistry, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences
- NATIONAL INSTITUTE OF GENERAL MEDICAL SCIENCES [P20GM103424] Funding Source: NIH RePORTER
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Cesium lead halide perovskite nanocrystals (NCs) possess excellent optical properties at visible wavelengths with great promise for applications in luminous display fields. We demonstrate a method to modify the surface ligand passivation of perovskite NCs for enhanced colloidal stability and emitting properties by incorporating didodecyl dimethyl ammonium bromide (DDAB). The photoluminescence quantum yield of the NC solution was improved to 96% from 70% and the perovskite film showed fewer trapped sites and enhanced carrier transport ability. The thus fabricated electroluminescent perovskite NC-LEDs exhibited a bright luminance of 11990 cd m(-2), corresponding to 4-times improved external quantum efficiency (EQE), compared to the control device using regular NCs without DDAB.
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