Journal
NANOSCALE
Volume 5, Issue 18, Pages 8711-8717Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3nr01608k
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Funding
- Priority Research Center Program [2012-0006682]
- Basic Science Research Program through the National Research Foundation of Korea [2012R1A1A2043731]
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The visible green and red upconversion emissions in Er3+/Yb3+ doped beta-NaGdF4 nanoparticles were enhanced by tridoping with Fe3+ ions (0-40 mol%). XRD, XPS, ICP-AES and EDS data demonstrated successful incorporation of Fe3+ ions in NaGdF4:Yb3+/Er3+ nanoparticles. The effect of Fe3+ tridoping on the upconversion luminescence in NaGdF4:Yb3+/Er3+ NPs was investigated in detail. The green and red emission intensities were enhanced by 34 and 30 times, respectively. The maximum emission was observed in a sample containing 30 mol% Fe3+ ions. A possible mechanism for the enhanced upconversion emission is proposed. In addition, a layer of silica was coated onto the surface of UCNPs to improve the biocompatibility. Folic acid was covalently linked to the silica coated UCNPs to form UCNP@SiO2-FA nanoprobes, which have been successfully applied to the fluorescent imaging HeLa cells.
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