4.8 Article

Silicon-Phosphorene Nanocavity-Enhanced Optical Emission at Telecommunications Wavelengths

Journal

NANO LETTERS
Volume 18, Issue 10, Pages 6515-6520

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acs.nanolett.8b03037

Keywords

silicon photonics; nanomaterials; phosphorene; silicon optical emission; two-dimensional materials; nanophotonics

Funding

  1. U.S. Department of Energy, Office of Science [DE-AC02-06CH11357]
  2. Argonne National Laboratory
  3. U.S. Department of Energy [DE-AC02-06CH11357]
  4. French RENATECH network
  5. Alexei Abrikosov Fellowship
  6. FACCTS Program (France and Chicago Collaborating in the Sciences) at the University of Chicago
  7. National Science Foundation [DMR-1505849]

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Generating and amplifying light in silicon (Si) continues to attract significant attention due to the possibility of integrating optical and electronic components in a single material platform. Unfortunately, silicon is an indirect band gap material and therefore an inefficient emitter of light. With the rise of integrated photonics, the search for silicon-based light sources has evolved from a scientific quest to a major technological bottleneck for scalable, CMOS-compatible, light sources. Recently, emerging two-dimensional materials have opened the prospect of tailoring material properties based on atomic layers. Few-layer phosphorene, which is isolated through exfoliation from black phosphorus (BP), is a great candidate to partner with silicon due to its layer-tunable direct band gap in the near-infrared where silicon is transparent. Here we demonstrate a hybrid silicon optical emitter composed of few-layer phosphorene nanomaterial flakes coupled to silicon photonic crystal resonators. We show single-mode emission in the telecommunications band of 1.55 mu m (E-g = 0.8 eV) under continuous wave optical excitation at room temperature. The solution-processed few-layer BP flakes enable tunable emission across a broad range of wavelengths and the simultaneous creation of multiple devices. Our work highlights the versatility of the Si-BP material platform for creating optically active devices in integrated silicon chips.

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